Controlling the carrier-envelope phase of Raman-generated periodic waveforms

Controlling the carrier-envelope phase of Raman-generated periodic waveforms
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We demonstrated control of the carrier-envelope phase of ultrashort periodic waveforms that are synthesized from a Raman-generated optical frequency comb. We generated the comb by adiabatically driving a molecular vibrational coherence with a beam at a fundamental frequency plus its second harmonic. Heterodyne measurements show that full interpulse phase locking of the comb components is realized.